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Assessment of Cs2HfCl6 crystal applicability as low-temperature scintillating bolometers by their thermodynamic characteristics

Dumoulin, L ; Giuliani, A ; Kandel, R ; Khalife, H ; Kuznetsov, S V ; Nagorny, S S ; Nahorna, V V ; Nishchev, K N ; Nones, C ; Olivieri, E ; Poda, D V ; Popov, P A ; Pynenkov, A A ; Stenning, G ; Wang, P ; Zolotarova, A S

J.Mater.Chem. C, 2022-01, Vol.10 (13), p.5218-5229 [Periódico revisado por pares]

Cambridge: Royal Society of Chemistry

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Título:
Assessment of Cs2HfCl6 crystal applicability as low-temperature scintillating bolometers by their thermodynamic characteristics
Autor: Dumoulin, L ; Giuliani, A ; Kandel, R ; Khalife, H ; Kuznetsov, S V ; Nagorny, S S ; Nahorna, V V ; Nishchev, K N ; Nones, C ; Olivieri, E ; Poda, D V ; Popov, P A ; Pynenkov, A A ; Stenning, G ; Wang, P ; Zolotarova, A S
Assuntos: Cryogenic temperature ; Crystals ; Detectors ; Gamma irradiation ; Infrared spectra ; Low temperature ; Near infrared radiation ; Phonons ; Physics ; Refractivity ; Room temperature ; Temperature ; Thermal conductivity ; Thermal expansion ; Thermodynamic properties ; Thermodynamics
É parte de: J.Mater.Chem. C, 2022-01, Vol.10 (13), p.5218-5229
Descrição: The first study of some thermodynamic properties of a Cs2HfCl6 (CHC) scintillating crystal has been performed in a wide temperature range of 5–300 K. The CHC crystal exhibits a high thermal expansion coefficient (5.17 × 10−5 at 171 K), along with an extremely low heat conductivity (1.710 W m−1 K−1 at 50 K). A high heat capacity (1.22 J kg−1 K−1 at 3.8 K) along with a drastically low free mean path for phonons (about 26 Å) at temperatures around 50 K makes the CHC crystal unsuitable as a target material for cryogenic detectors. The results of the first operation of the CHC crystal as a cryogenic detector at sub-Kelvin temperatures clearly show the unfavorable phonon propagation properties of the material. On the other hand, the CHC crystal demonstrates excellent scintillating characteristics with a relatively high light yield under gamma irradiation (the detected signal is about 5200 photons per MeV). The refractive index within the (1.66–1.67) interval for light in visible and near-infrared spectral ranges was measured at room temperature. A cost- and time-effective approach for new crystalline material characterization as a target for cryogenic detectors based on the evaluation of the thermodynamic properties of the material is proposed.
Editor: Cambridge: Royal Society of Chemistry
Idioma: Inglês

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Assessment of Cs2HfCl6 crystal applicability as low-temperature scintillating bolometers by their thermodynamic characteristics

Dumoulin, L ; Giuliani, A ; Kandel, R ; Khalife, H ; Kuznetsov, S V ; Nagorny, S S ; Nahorna, V V ; Nishchev, K N ; Nones, C ; Olivieri, E ; Poda, D V ; Popov, P A ; Pynenkov, A A ; Stenning, G ; Wang, P ; Zolotarova, A S

Cambridge: Royal Society of Chemistry

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