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Molecular magnetism, quo vadis? A historical perspective from a coordination chemist viewpoint

Ferrando-Soria, Jesús ; Vallejo, Julia ; Castellano, María ; Martínez-Lillo, José ; Pardo, Emilio ; Cano, Joan ; Castro, Isabel ; Lloret, Francesc ; Ruiz-García, Rafael ; Julve, Miguel

Coordination chemistry reviews, 2017-05, Vol.339, p.17-103 [Periódico revisado por pares]

Elsevier B.V

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  • Título:
    Molecular magnetism, quo vadis? A historical perspective from a coordination chemist viewpoint
  • Autor: Ferrando-Soria, Jesús ; Vallejo, Julia ; Castellano, María ; Martínez-Lillo, José ; Pardo, Emilio ; Cano, Joan ; Castro, Isabel ; Lloret, Francesc ; Ruiz-García, Rafael ; Julve, Miguel
  • Assuntos: Coordination chemistry ; Molecular magnetism ; Molecular spintronics ; Quantum computation ; Single molecules
  • É parte de: Coordination chemistry reviews, 2017-05, Vol.339, p.17-103
  • Descrição: [Display omitted] •Coordination chemistry approach from molecular magnetism to molecular spintronics and quantum computation.•Electron exchange and double exchange in homo- and heterovalent dinuclear complexes.•Spin crossover and valence tautomerism in mono-, di- and tetranuclear complexes.•Magnetic anisotropy and spin dynamics in metal clusters and coordination polyhedra.•Spin dynamics and quantum coherence in mononuclear complexes and metal rings. Molecular magnetism has travelled a long way from the pioneering studies on electron exchange and double exchange or spin crossover and valence tautomerism in small oligonuclear complexes, from mono- to di- and tetranuclear species, to the current investigations about magnetic anisotropy and spin dynamics or quantum coherence of simple mono- or large polynuclear complexes, behaving as switchable bistable molecular nanomagnets for potential applications in information data storage and processing. In this review, we focus on the origin and development of the research in the field of molecular magnetism from a coordination chemistry viewpoint, which dates back to the establishment of magnetochemistry as a novel discipline among the molecular sciences. This overview is conceived as an attempt to orientate coordination chemists regarding their role in the future direction that molecular magnetism will undergo in its further evolution toward molecular spintronics and quantum computation. A particular emphasis will be given to some selected recent advances in single-molecule spintronic circuitry and quantum computing devices based on the large class of multiresponsive and multifunctional magnetic metal complexes to stimulate the progress in the field of molecular magnetism.
  • Editor: Elsevier B.V
  • Idioma: Inglês
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  • Realização: ABCD-USP USP   Logos de Redes Sociais: Freepik

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