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Liquid-like thermal conduction in intercalated layered crystalline solids

Li, B ; Wang, H ; Kawakita, Y ; Zhang, Q ; Feygenson, M ; Yu, H. L ; Wu, D ; Ohara, K ; Kikuchi, T ; Shibata, K ; Yamada, T ; Ning, X. K ; Chen, Y ; He, J. Q ; Vaknin, David ; Wu, R. Q ; Nakajima, K ; Kanatzidis, M. G

Iowa State University Digital Repository 2018

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  • Título:
    Liquid-like thermal conduction in intercalated layered crystalline solids
  • Autor: Li, B ; Wang, H ; Kawakita, Y ; Zhang, Q ; Feygenson, M ; Yu, H. L ; Wu, D ; Ohara, K ; Kikuchi, T ; Shibata, K ; Yamada, T ; Ning, X. K ; Chen, Y ; He, J. Q ; Vaknin, David ; Wu, R. Q ; Nakajima, K ; Kanatzidis, M. G
  • Assuntos: Biological and Chemical Physics ; Condensed Matter Physics ; Materials Chemistry ; Physical Chemistry ; Thermodynamics
  • Notas: Ames Laboratory Accepted Manuscripts
  • Descrição: As a generic property, all substances transfer heat through microscopic collisions of constituent particles1. A solid conducts heat through both transverse and longitudinal acoustic phonons, but a liquid employs only longitudinal vibrations2,3. As a result, a solid is usually thermally more conductive than a liquid. In canonical viewpoints, such a difference also serves as the dynamic signature distinguishing a solid from a liquid. Here, we report liquid-like thermal conduction observed in the crystalline AgCrSe2. The transverse acoustic phonons are completely suppressed by the ultrafast dynamic disorder while the longitudinal acoustic phonons are strongly scattered but survive, and are thus responsible for the intrinsically ultralow thermal conductivity. This scenario is applicable to a wide variety of layered compounds with heavy intercalants in the van der Waals gaps, manifesting a broad implication on suppressing thermal conduction. These microscopic insights might reshape the fundamental understanding on thermal transport properties of matter and open up a general opportunity to optimize performances of thermoelectrics.
  • Editor: Iowa State University Digital Repository
  • Data de criação/publicação: 2018
  • Idioma: Inglês
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  • Realização: ABCD-USP USP   Logos de Redes Sociais: Freepik

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