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Imaging molecular structure through femtosecond photoelectron diffraction on aligned and oriented gas-phase molecules

Boll, Rebecca ; Rouzée, Arnaud ; Adolph, Marcus ; Anielski, Denis ; Aquila, Andrew ; Bari, Sadia ; Bomme, Cédric ; Bostedt, Christoph ; Bozek, John D ; Chapman, Henry N ; Christensen, Lauge ; Coffee, Ryan ; Coppola, Niccola ; De, Sankar ; Decleva, Piero ; Epp, Sascha W ; Erk, Benjamin ; Filsinger, Frank ; Foucar, Lutz ; Gorkhover, Tais ; Gumprecht, Lars ; Hömke, André ; Holmegaard, Lotte ; Johnsson, Per ; Kienitz, Jens S ; Kierspel, Thomas ; Krasniqi, Faton ; Kühnel, Kai-Uwe ; Maurer, Jochen ; Messerschmidt, Marc ; Moshammer, Robert ; Müller, Nele L. M ; Rudek, Benedikt ; Savelyev, Evgeny ; Schlichting, Ilme ; Schmidt, Carlo ; Scholz, Frank ; Schorb, Sebastian ; Schulz, Joachim ; Seltmann, Jörn ; Stener, Mauro ; Stern, Stephan ; Techert, Simone ; Thøgersen, Jan ; Trippel, Sebastian ; Viefhaus, Jens ; Vrakking, Marc ; Stapelfeldt, Henrik ; Küpper, Jochen ; Ullrich, Joachim ; Rudenko, Artem ; Rolles, Daniel

Faraday discussions, 2014-01, Vol.171, p.57-8 [Periódico revisado por pares]

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Título:
Imaging molecular structure through femtosecond photoelectron diffraction on aligned and oriented gas-phase molecules
Autor: Boll, Rebecca ; Rouzée, Arnaud ; Adolph, Marcus ; Anielski, Denis ; Aquila, Andrew ; Bari, Sadia ; Bomme, Cédric ; Bostedt, Christoph ; Bozek, John D ; Chapman, Henry N ; Christensen, Lauge ; Coffee, Ryan ; Coppola, Niccola ; De, Sankar ; Decleva, Piero ; Epp, Sascha W ; Erk, Benjamin ; Filsinger, Frank ; Foucar, Lutz ; Gorkhover, Tais ; Gumprecht, Lars ; Hömke, André ; Holmegaard, Lotte ; Johnsson, Per ; Kienitz, Jens S ; Kierspel, Thomas ; Krasniqi, Faton ; Kühnel, Kai-Uwe ; Maurer, Jochen ; Messerschmidt, Marc ; Moshammer, Robert ; Müller, Nele L. M ; Rudek, Benedikt ; Savelyev, Evgeny ; Schlichting, Ilme ; Schmidt, Carlo ; Scholz, Frank ; Schorb, Sebastian ; Schulz, Joachim ; Seltmann, Jörn ; Stener, Mauro ; Stern, Stephan ; Techert, Simone ; Thøgersen, Jan ; Trippel, Sebastian ; Viefhaus, Jens ; Vrakking, Marc ; Stapelfeldt, Henrik ; Küpper, Jochen ; Ullrich, Joachim ; Rudenko, Artem ; Rolles, Daniel
Assuntos: Angular distribution ; Atom and Molecular Physics and Optics ; Atom- och molekylfysik och optik ; Diffraction ; Femtosecond ; Free electron lasers ; Fysik ; Lasers ; Natural Sciences ; Naturvetenskap ; Photoelectrons ; Physical Sciences ; Spectra ; X-rays
É parte de: Faraday discussions, 2014-01, Vol.171, p.57-8
Notas: ObjectType-Article-1
SourceType-Scholarly Journals-1
ObjectType-Feature-2
content type line 23
Descrição: This paper gives an account of our progress towards performing femtosecond time-resolved photoelectron diffraction on gas-phase molecules in a pump-probe setup combining optical lasers and an X-ray free-electron laser. We present results of two experiments aimed at measuring photoelectron angular distributions of laser-aligned 1-ethynyl-4-fluorobenzene (C 8 H 5 F) and dissociating, laser-aligned 1,4-dibromobenzene (C 6 H 4 Br 2 ) molecules and discuss them in the larger context of photoelectron diffraction on gas-phase molecules. We also show how the strong nanosecond laser pulse used for adiabatically laser-aligning the molecules influences the measured electron and ion spectra and angular distributions, and discuss how this may affect the outcome of future time-resolved photoelectron diffraction experiments.
Editor: England
Idioma: Inglês

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Imaging molecular structure through femtosecond photoelectron diffraction on aligned and oriented gas-phase molecules

England

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